Volume 65 (2020): Issue 3 (September 2020)

The possibility of preparing fission chambers for the experimental determination of subcriticality without time-consuming corrections has been presented. The reactor detectors set consists of monoisotopic chambers. Each chamber is intended for a specific position in the system. Individual weights, rated a priori for all detectors in their positions, allow for quick calculation of whole system subcriticality. The inconveniences related to the spatial effect are minimized. This is achieved by computational simulation of the area method results, for each detector position and all possible fissionable and fissile nuclides. Next, one nuclide is selected, specific for the given position, presenting the smallest difference from the MCNP KCODE precisely estimated kkcode. The case study is made using the model of VENUS-F core.

X-rays application for radiation processing was introduced to the industrial practice, and in some circumstances is found to be more economically competitive, and offer more flexibility than gamma sources. Recent progress in high-power accelerators development gives opportunity to construct and apply reliable high-power electron beam to X-rays converters for the industrial application. The efficiency of the conversion process depends mainly on electron energy and atomic number of the target material, as it was determined in theoretical predictions and confirmed experimentally. However, the lower price of low-energy direct accelerators and their higher electrical efficiency may also have certain influence on process economy. There are number of auxiliary parameters that can effectively change the economical results of the process. The most important ones are as follows: average beam power level, spare part cost, and optimal shape of electron beam and electron beam utilization efficiency. All these parameters and related expenses may affect the unit cost of radiation facility operation and have a significant influence on X-ray process economy. The optimization of X-rays converter construction is also important, but it does not depend on the type of accelerator. The article discusses the economy of radiation processing with high-intensity of X-rays stream emitted by conversion of electron beams accelerated in direct accelerator (electron energy 2.5 MeV) and resonant accelerators (electron energy 5 MeV and 7.5 MeV). The evaluation and comparison of the costs of alternative technical solutions were included to estimate the unit cost of X-rays facility operation for average beam power 100 kW.

Source term is the amount of radionuclide activity, measured in becquerels, released to the atmosphere from a nuclear reactor, together with the plume composition, over a specific period. It is the basis of radioprotection-related calculation. Usually, such computations are done using commercial codes; however, they are challenging to be used in the case of the MARIA reactor due to its unique construction. Consequently, there is a need to develop a method that will be able to deliver useful results despite the complicated geometry of the reactor site. Such an approach, based upon the Bateman balance equation, is presented in the article, together with the results of source term calculation for the MARIA reactor. Additionally, atmospheric dispersion of the radionuclides, analysed with the Gauss plume model with dry deposition, is presented.

The city of Krakow located in southern Poland ranks among the most polluted urban agglomerations in Europe. There are persisting controversies with respect to impact of different pollution sources operating in Krakow agglomeration on air quality within the city. The presented pilot study was aimed at exploring the possibilities offered by elemental and carbon isotope composition of total suspended particulate matter (TSPM) for better characterization of its sources in Krakow atmosphere. The analyses of carbon isotope composition of total carbon in the investigated TSPM samples were supplemented by parallel analyses of radiocarbon content in atmospheric carbon dioxide (CO₂). This study revealed large seasonal variability of carbon isotope composition in the analysed TSPM samples. This large variability reflects seasonally varying contribution of different sources of fossil and modern carbon to the TSPM pool. The elemental composition of TSPM also reveals distinct seasonal variability of the analysed elements, reflecting varying mixture of natural and anthropogenic sources of those elements. A linear relationship between the fossil carbon load in the TSPM samples and the fossil carbon load in the atmospheric CO₂ was found, pointing to the presence of additional source of anthropogenic carbonaceous particles not associated with burning of fossil fuels. Wearing of tyres and asphalt pavement is most probably the main source of such particles.

This paper presents the results of long-term investigations of ¹³⁷Cs and ¹³⁴Cs activity concentrations in drinking water in the city of Zagreb for the period 1987–2018. The highest activity concentrations of both radio-nuclides were measured in 1987, decreasing exponentially ever since, while ¹³⁴Cs in several subsequent years fell under the detection limit. After the Fukushima Daiichi accident in 2011, the presence of ¹³⁴Cs in drinking water was detected again. The environmental residence time for ¹³⁷Cs was estimated to be 8.1 years in drinking water and 5.7 years in fallout. The correlation between ¹³⁷Cs in fallout and in drinking water is very good, and this indicates that fallout is the main source of water contamination. The observed ¹³⁴Cs/¹³⁷Cs activity ratio in drinking water for the post-Chernobyl period was similar to the ratio found in other environmental samples. The estimation of annual effective doses received by the adult members of the Croatian population due to the intake of radiocaesium in drinking water showed quite small doses of 0.28 μSv in 1987 decreasing to 2.5 nSv in 2018, which indicated that drinking water was not a critical pathway for the transfer of radiocaesium to humans.